Data-Driven Photoluminescence Tuning in Eu2+-Doped Phosphors | Научно-инновационный портал СФУ

Data-Driven Photoluminescence Tuning in Eu2+-Doped Phosphors

Тип публикации: статья из журнала

Год издания: 2020

Идентификатор DOI: 10.1021/acs.jpclett.0c01471

Аннотация: Discovery of rare earth phosphors has generally relied on the chemical intuition and time-intensive trial-and-error synthesis; therefore, finding new materials assisted by data-driven computations is urgent. Herein, we utilize a regression model to predict the emission wavelengths of Eu2+-doped phosphors by revealing the relationships between the crystal structure and luminescence property. The emission wavelengths of [Rb(1-x)K(x)]3LuSi2O7:Eu2+ (0 ≤ x ≤ 1) phosphors, as examples for the data-driven photoluminescence tuning, are successfully predicted on the basis of the existing data of only eight systems, also consistent with the experimental results. These phosphors can be excited by blue light and exhibit broad-band red and near-infrared emission ranging from 619 to 737 nm. These findings in Eu2+-doped silicate phosphors indicate that data-driven computations through the regression mode would have bright application in discovering novel phosphors with a target emission wavelengths.

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Издание

Журнал: The journal of physical chemistry letters

Выпуск журнала: Vol. 11, Is. 14

Номера страниц: 5680-5685

ISSN журнала: 19487185

Авторы

  • Lai Shunqi (South China Univ Technol, Sch Mat Sci & Engn, State Key Lab Luminescent Mat & Devices, Guangdong Prov Key Lab Fiber Laser Mat & Appl Tec, Guangzhou 510641, Peoples R China)
  • Zhao Ming (South China Univ Technol, Sch Mat Sci & Engn, State Key Lab Luminescent Mat & Devices, Guangdong Prov Key Lab Fiber Laser Mat & Appl Tec, Guangzhou 510641, Peoples R China; Univ Sci & Technol Beijing, Sch Mat Sci & Engn, Beijing Municipal Key Lab New Energy Mat & Techno, Beijing 100083, Peoples R China)
  • Qiao Jianwei (South China Univ Technol, Sch Mat Sci & Engn, State Key Lab Luminescent Mat & Devices, Guangdong Prov Key Lab Fiber Laser Mat & Appl Tec, Guangzhou 510641, Peoples R China; Univ Sci & Technol Beijing, Sch Mat Sci & Engn, Beijing Municipal Key Lab New Energy Mat & Techno, Beijing 100083, Peoples R China)
  • Molokeev Maxim S. (RAS, Kirensky Inst Phys, Lab Crystal Phys, Fed Res Ctr KSC SB, Krasnoyarsk 660036, Russia; Siberian Fed Univ, Krasnoyarsk 660041, Russia; Far Eastern State Transport Univ, Dept Phys, Khabarovsk 680021, Russia)
  • Xia Zhiguo (South China Univ Technol, Sch Mat Sci & Engn, State Key Lab Luminescent Mat & Devices, Guangdong Prov Key Lab Fiber Laser Mat & Appl Tec, Guangzhou 510641, Peoples R China; Univ Sci & Technol Beijing, Sch Mat Sci & Engn, Beijing Municipal Key Lab New Energy Mat & Techno, Beijing 100083, Peoples R China)

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